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We experimentally isolate, characterize and coherently control up to sixindividual nuclear spins that are weakly coupled to an electron spin indiamond. Our method employs multi-pulse sequences on the electron spin thatresonantly amplify the interaction with a selected nuclear spin and at the sametime dynamically suppress decoherence caused by the rest of the spin bath. Weare able to address nuclear spins with interaction strengths that are an orderof magnitude smaller than the electron spin dephasing rate. Our results providea route towards tomography with single-nuclear-spin sensitivity and greatlyextend the number of available quantum bits for quantum information processingin diamond.

Detection and control of individual nuclear spins using a weakly coupled electron spin