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Parametrized crystal-field analyses are presented for both the six and sevenfold coordinated, C$_{1}$ symmetry Sm$^{3+}$ centers in Y$_{2}$SiO$_{5}$, basedon extensive spectroscopic data spanning the infrared to optical regions. Lasersite-selective excitation and fluorescence spectroscopy as well as Zeemanabsorption spectroscopy performed along multiple crystallographic directionshas been utilised, in addition to previously determined $g$ tensors for the$^{6}$H$_{5/2}$Z$_{1}$ and $^{4}$G$_{5/2}$A$_{1}$ states. The resultantanalyses give good approximation to the experimental energy levels and magneticsplittings, yielding crystal-field parameters consistent with the few otherlanthanide ions for which such analyses are available.

journal of physics. condensed matter

Reproduction of the electronic and magnetic structure of the low  symmetry sites of Y$_{2}$SiO$_{5}$ doped with Sm$^{3+}$ via a parameterized  crystal-field model