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K(BEDT-TTF)2Cu(NCS)2 has been investigated by Raman scattering in both bulkand nanoparticle compounds. Phonon modes from 20 to 1600 cm-1 have beenassigned. Focusing on the unexplored low frequency phonons, a plateau infrequencies is observed in the bulk phonons between 50 and 100 K and assignedto the signature of the bad metal phase. Nanoparticles of K(BEDT-TTF)2Cu(NCS)2exhibit anomalies at 50 K associated to the crossover from a bad metal to aFermi liquid whose origins are discussed.

journal of physics. condensed matter

Possible observation of the signature of the bad metal phase and its  crossover to a Fermi liquid in K(BEDT-TTF)2Cu(NCS)2 bulk and nanoparticles by  Raman scattering