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Using combined magnetometry and ferromagnetic resonance studies, it is shownthat introduction of a hydrocarbon cover layer leads to an increase of thecontribution of the surface anisotropy to the effective magnetic anisotropyenergy of hexagonal close-packed 0001 cobalt films, largely enhancing theperpendicular anisotropy. Due to a weak electronic interaction of the organicmolecules with the Co atoms, an increase of surface anisotropy could beexplained by the presence of an electric field at the organic-material/Cointerface and by modification of surface atoms charge configuration.

Impact of organic capping layer on the magnetic anisotropy of ultrathin Co films