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We develop a Magnetic Cluster Expansion (MCE) model for binary bcc and fccFe-Cr alloys, as well as for fcc Fe-Ni alloys, and apply it to theinvestigation of magnetic properties of these alloys over a broad interval ofconcentrations, and over a broad interval of temperatures extending well over1000 K. We show how an MCE-based Monte Carlo study describes the magneticproperties of these alloys, for example the composition and microstructuredependence of the Curie temperature, the non-collinearity of magneticstructures found in bcc Fe-Cr alloys, phase transitions between bcc and fcc inFe-Cr, and the enthalpy of mixing of Fe-Ni alloys. The results of simulationsare in excellent agreement with experimental observations.

A novel Monte Carlo model and simulations of magnetic alloys for nuclear applications