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Quantitative two-photon absorption (2PA) cross section and 2PA spectrum measurements were used to determine the molecular electric dipole change in the metal-to-ligand charge-transfer transition of ruthenium(II) tris-complexes of 2,2’-bipyridine ([Ru(bpy) 3 ] 2+ ) and 1,10-phenanthroline ([Ru(phen) 3 ] 2+ ) in several solvents.

Quantitative description of MLCT transitions in ruthenium polypyridyl complexes probed by two-photon absorption spectroscopy