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Ultrafast dynamics of photoinduced processes in [Fe(CO)5]n clusters and free Fe(CO)5 molecules excited by resonant femtosecond IR radiation (λ ~ 5 μm) were studied in a molecular beam. Using a pump-probe teqnique characteristic rates of these processes were obtained and theoretically analyzed

Ultrafast dynamics of photoprocesses induced by femtosecond IR laser radiation in iron pentacarbonyl molecules and clusters