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Graphene based two-dimensional (2D) van der Waals (vdW) materials have attracted enormous attention because of their extraordinary physical properties. In this study, we explore the temperature and interlayer coupling induced thermal transport across the graphene/2D-SiC vdW interface using non-equilibrium molecular dynamics and transient pump probe methods. We find that the in-plane thermal conductivity  κ  deviates slightly from the 1/ T  law at high temperatures. A tunable  κ  is found with the variation of the interlayer coupling strength χ .  The interlayer thermal resistance  R  across graphene/2D-SiC interface reaches 2.71    $$\times$$  × 10 –7    $${\text{Km}}^{2} /{\text{W}}$$  Km 2 / W at room temperature and χ = 1, and it reduces steadily with the elevation of system temperature and χ, demonstrating around 41% and 56% reduction with increasing temperature to 700 K and a χ of 25, respectively. We also elucidate the heat transport mechanism by estimating the in-plane and out-of-plane phonon modes. Higher phonon propagation possibility and Umklapp scattering across the interface at high temperatures and increased χ lead to the significant reduction of  R . This work unveils the mechanism of heat transfer and interface thermal conductance engineering across the graphene/2D-SiC vdW heterostructure.

Temperature and interlayer coupling induced thermal transport across graphene/2D-SiC van der Waals heterostructure