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Highlights2D Ti 3 C 2 T  x   MXene nanosheets with high electrical conductivity and mobility were employed as a nanosized additive to prepare 2D perovskite films.    Doping of Ti 3 C 2 T  x   nanosheets can passivate the defects on the perovskite films surface and accelerate charge transfer process in vertical direction.    Enhanced crystallinity and orientation of the perovskite films result in a significant increase in short-circuit current density and power conversion efficiency.Supplementary Information  The online version contains supplementary material available at 10.1007/s40820-021-00602-w.

Efficient Two-Dimensional Perovskite Solar Cells Realized by Incorporation of Ti3C2Tx MXene as Nano-Dopants