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HighlightsThe self-assembled louver-like P-doped carbon nitride (L-PCN) nanowires is firstly constructed.    L-PCN nanowires show efficient charge transport, as demonstrated by experimental and theoretical approach.    L-PCN nanowires exhibit significantly boosted HER activity of 1,872.9 μmol h −1  g −1  ( λ  > 420 nm).Electronic supplementary material  The online version of this article (10.1007/s40820-020-0399-1) contains supplementary material, which is available to authorized users.

Hierarchical Self-assembly of Well-Defined Louver-Like P-Doped Carbon Nitride Nanowire Arrays with Highly Efficient Hydrogen Evolution