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HighlightsUltrathin (< 600 nm) and defect-free leaf-like UiO-66-SO 3 H membranes were fabricated via in situ smart growth.    The sulfonated angstrom-sized ion transport channels in the membranes could accelerate the cation permeation (~ 3×  faster than non-functionalized UiO-66 membrane) and achieve a high ion selectivity (Na + /Mg 2+  > 140).Electronic supplementary material  The online version of this article (10.1007/s40820-020-0386-6) contains supplementary material, which is available to authorized users.

Engineering Leaf-Like UiO-66-SO3H Membranes for Selective Transport of Cations