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HighlightsThe unique hairball-like VS 4  composed of spiral nanowires was successively constructed through a one-step hydrothermal method.    The prepared hairball-like VS 4  exhibits high capacity and long cycle stability for Na +  storage at room temperature, and it can tolerate drastic temperature changes.    The ex situ characterization and electrochemical kinetic analysis reveal that the storage mechanisms of VS 4  changed with the increase in the number of cycles.Electronic supplementary material  The online version of this article (10.1007/s40820-020-0377-7) contains supplementary material, which is available to authorized users.

Three-Dimensional Self-assembled Hairball-Like VS4 as High-Capacity Anodes for Sodium-Ion Batteries