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HighlightsN, O co-doped graphene layered block (NOGB) was prepared as sulfur host for lithium–sulfur batteries.    The NOGB/S shows good rate performance due to robust electrochemical kinetics.    The strong physicochemical confinement leads to an improved cycling stability.Electronic supplementary material  The online version of this article (10.1007/s40820-020-00477-3) contains supplementary material, which is available to authorized users.

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Sandwiching Sulfur into the Dents Between N, O Co-Doped Graphene Layered Blocks with Strong Physicochemical Confinements for Stable and High-Rate Li–S Batteries