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HighlightsThree-dimensional phosphorus@graphene is established as a negative electrode and Ni 2 P as a positive electrode for asymmetric supercapacitor.    The supercapacitor shows higher performance than those of all Ni 2 P-based electrodes, which has an extended operating voltage window of 1.6 V, energy density of 41.66 Wh Kg −1  and rate capability of up to 88% after 5000 cycles.Electronic supplementary material  The online version of this article (10.1007/s40820-019-0360-3) contains supplementary material, which is available to authorized users.

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Newly Design Porous/Sponge Red Phosphorus@Graphene and Highly Conductive Ni2P Electrode for Asymmetric Solid State Supercapacitive Device With Excellent Performance